Articles | Volume 2, issue 1
https://doi.org/10.5194/ar-2-49-2024
© Author(s) 2024. This work is distributed under the Creative Commons Attribution 4.0 License.
Opinion: A paradigm shift in investigating the general characteristics of atmospheric new particle formation using field observations
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- Final revised paper (published on 27 Mar 2024)
- Preprint (discussion started on 21 Dec 2023)
Interactive discussion
Status: closed
Comment types: AC – author | RC – referee | CC – community | EC – editor | CEC – chief editor
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- RC1: 'Comment on ar-2023-19', Anonymous Referee #1, 17 Jan 2024
- RC2: 'Comment on ar-2023-19', Anonymous Referee #2, 31 Jan 2024
- AC1: 'Comment on ar-2023-19', Markku Kulmala, 14 Feb 2024
Peer review completion
AR – Author's response | RR – Referee report | ED – Editor decision | EF – Editorial file upload
AR by Markku Kulmala on behalf of the Authors (14 Feb 2024)
Author's tracked changes
Manuscript
EF by Polina Shvedko (16 Feb 2024)
Author's response
ED: Publish as is (17 Feb 2024) by Daniele Contini
AR by Markku Kulmala on behalf of the Authors (18 Mar 2024)
Manuscript
In this MS the authors propose a new way to study atmospheric NPF, in a more statistical sense. Starting from data collected in field observations, this method aims to create a probability distribution of particle formation (JC) and growth rates (GR) to obtain statistical information on the intensity of NPF. Instead of making the traditional classification of NPF, between event and non-event, and analysing only a sub-set of data, this method uses a continuous approach by analysing all available days. The analysis is performed on particle and ion number concentrations in the size range of particles (2.5-5 nm) or intermediate ions (2-7 nm). Although this is an innovative method that can quantify both local and regional NPF contributions to the total particle number concentrations in the atmosphere, it is very limited. It can only be used if the measurement site has adequate instrumentation to measure the sub-5 nm size range needed to apply the method.
Therefore, the proposed approach can represent a useful but complementary tool to the traditional NPF event analysis.
I think that this is an important work since NPF is a topic of current interest and the authors are well-informed and experienced about it. Furthermore, this work is well written, offering a clear exposition of the topic. Therefore, this manuscript has enough quality to be published in this journal.
I just have few suggestions to the authors:
Line 25: the first sentence of the abstract “Atmospheric new particle formation (NPF), together with secondary production”, seems to mean that the NPF is not from secondary origin.
Line 66: it is not clear “in terms of discrete”.
Line 112: Please explain “sizes relevant to climate or air quality”.