Preprints
https://doi.org/10.5194/ar-2025-19
https://doi.org/10.5194/ar-2025-19
23 Jun 2025
 | 23 Jun 2025
Status: this preprint is currently under review for the journal AR.

A Cross-Correlation Based Method for Determining Size-Resolved Particle Growth Rates

Janne Lampilahti, Pauli Paasonen, Santeri Tuovinen, Katrianne Lehtipalo, Veli-Matti Kerminen, and Markku Kulmala

Abstract. The particle growth rate (GR) is a key parameter in aerosol dynamics and plays a crucial role in understanding atmospheric new particle formation and its effects. A fast, robust and reproducible calculation of GRs from aerosol number-size distribution data remains a challenge. In this study, we introduce a new method that we call the maximum correlation method for calculating particle and ion GRs from number-size distributions. We employed this novel method to calculate GRs from Hyytiälä, Finland using 14 years of ion and total particle size distribution data and compared our results against previous studies that used conventional methods for calculating the GRs. We found that our method compares well against the published data and reproduces the seasonal variability and size-dependent trends in the GRs. The maximum correlation method enables fast and repeatable GR calculations from large aerosol datasets, which facilitates the systematic incorporation of GR analysis into new particle formation studies.

Competing interests: Markku Kulmala is a member of the editorial board of Aerosol Research.

Publisher's note: Copernicus Publications remains neutral with regard to jurisdictional claims made in the text, published maps, institutional affiliations, or any other geographical representation in this preprint. The responsibility to include appropriate place names lies with the authors.
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Janne Lampilahti, Pauli Paasonen, Santeri Tuovinen, Katrianne Lehtipalo, Veli-Matti Kerminen, and Markku Kulmala

Status: open (until 04 Aug 2025)

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Janne Lampilahti, Pauli Paasonen, Santeri Tuovinen, Katrianne Lehtipalo, Veli-Matti Kerminen, and Markku Kulmala

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Dataset for "A Cross-Correlation-Based Method for Determining Size-Resolved Particle Growth Rates" Janne Lampilahti, Pauli Paasonen, Santeri Tuovinen, Katrianne Lehtipalo, Veli-Matti Kerminen, Markku Kulmala https://doi.org/10.5281/zenodo.15648698

Janne Lampilahti, Pauli Paasonen, Santeri Tuovinen, Katrianne Lehtipalo, Veli-Matti Kerminen, and Markku Kulmala
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Short summary
We developed a new automated method for calculating aerosol particle growth rates. Based on 14 years of measurements from Hyytiälä, Finland, the method produces results comparable to conventional approaches, while offering improved speed and ease of use.
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